Title: Atomic layer graphene as saturable absorber for ultrafast pulsed lasers

The optical conductance of monolayer graphene is defined solely by the fine structure constant, α = e²/hc (where e is the electron charge, h is Dirac’s constant and c is the speed of light). The absorbance has been predicted to be independent of frequency. In principle, the interband optical absorption in zero-gap graphene could be saturated readily under strong excitation due to Pauli blocking. Here, we demonstrate the use of atomic layer graphene as saturable absorber in a mode-locked fiber laser for the generation of ultrashort soliton pulses (756 fs) at the telecommunication band. The modulation depth can be tuned in a wide range from 66.5% to 6.2% by varying the thickness of graphene. Our results suggest that ultrathin graphene films are potentially useful as optical elements in fiber lasers. Graphene as a laser mode locker can have many merits such as lower saturation intensity, ultrafast recovery time, tunable modulation depth and wideband tuneability.

DOI: 10.1002/adfm.200901007