2024年5月10日，Elsevier 旗下top期刊《Journal of Colloid and Interface Science》在线发表了云南师范大学化学与化工学院高端引进人才赵学博士、张义成博士、云南大学胡广志、浙江海洋大学周英堂教授等团队合作的最新研究成果《Pomelo peel biomass derived highly active advanced-oxidation-process catalyst:Complete elimination of organic pollutants》。第一作者单位为云南师范大学化学化工学院，浙江海洋大学为共同第一作者单位。云南师范大学化学化工学院张义成、赵学、云南大学胡广志教授和浙江海洋大学周英堂教授为共同通讯作者。文章报道了柚皮生物质衍生的高活性高级氧化催化消除有机污染物的研究，这是赵学博士今年以来的第四篇TOP期刊文章。

Abstract

The advanced oxidation process (AOPs) is playing an important role in the elimination of hazardous organic pollutants, but the development of inexpensive and highly active advanced catalysts is facing challenges. In this study, a low-cost and readily available agricultural waste resource pomelo peel-flesh (PPF) biomass was used as the basic raw material, and the uniformly dispersed small cobalt nanoparticles were effectively anchored in the biochar derived from pomelo peel-flesh (BDPPF) by impregnation adsorption/complexation combined with heat treatment. Co/BDPPF (BDPPF embedded with Co) can effectively activate peroxymonosulfate (PMS) to SO4·-, ·OH and 1O2 reactive oxygen species, and achieve nearly 100% degradation of tetracycline persistent organic pollutant. Co/BDPPF can not only degrade tetracycline efficiently in complex water environment, but also degrade most organic pollutants universally, and has long-term stability, which solves the problem of poor universality and stability of heterogeneous catalysts to a certain extent. Importantly, Co/BDPPF derived from waste biomass was also innovatively designed as the core of an integrated continuous purification device to achieve continuous purification of organic wastewater. In this study, agricultural waste resources were selected as biomass raw materials to achieve efficient capture of Co2+, and finally developed advanced AOPs catalyst with excellent performance to achieve the purification of organic wastewater. It also provides a promising solution for the preparation of simple, low-cost, large-scale production of AOPs catalysts that can be put into actual production.

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