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W6.48 Opens a Gate for a Continuous Intrinsic Water Pathway

已有 2769 次阅读 2014-11-18 19:33 |个人分类:科研笔记|系统分类:科研笔记

Angew Chem  Int Edit .   17/11/2014; 53(1-5).   DOI: 10.1002/anie.201409679          

Shuguang Yuan*, Zhenquan Hu, Slawomir Filipek, Horst Vogel*

fulltext: http://onlinelibrary.wiley.com/enhanced/doi/10.1002/anie.201409679/


ABSTRACT The question how G-protein-coupled receptors transduce an extracellular signal by a sequence of transmembrane conformational transitions into an intracellular response remains to be solved at molecular detail. Herein, we use molecular dynamics simulations to reveal distinct conformational transitions of the adenosine A2A receptor, and we found that the conserved W2466.48 residue in transmembrane helix TM6 performs a key rotamer toggle switch. Agonist binding induces the sidechain of W2466.48 to fluctuate between two distinct conformations enabling the diffusion of water molecules from the bulk into the center of the receptor. After passing the W2466.48 gate, the internal water molecules induce another conserved residue, Y2887.53, to switch to a distinct rotamer conformation establishing a continuous transmembrane water pathway. Further, structural changes of TM6 and TM7 induce local structural changes of the adjacent lipid bilayer.





https://blog.sciencenet.cn/blog-355217-844399.html

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