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ICM第2期图文目录 | Volume 1,Issue 2

已有 999 次阅读 2023-6-2 10:08 |个人分类:ICM文章|系统分类:论文交流

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Industrial Chemistry & Materials Volume 1,Issue 2 文章正式出版啦!本期文章共收录文章9篇,包括研究论文4篇,综述5篇。欢迎广大读者阅读、下载和分享!

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  • 本期封面

  Front cover  

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本期封面文章来自德国莱布尼茨催化研究所、德国科学院院士Matthias Beller教授团队综述:Industrially Applied and Relevant Transformations of 1,3-Butadiene using Homogeneous Catalysts。本图以1,3-丁二烯的工业转化为核心,生动展示了通过均相催化将其转化为1-辛烯、1-辛醇、己二腈等功能化学品的过程。其中,均相催化剂充当关键的转化媒介。随着分子转化,其经济价值显著提升,与文章阐述的通过化工过程设计从分子层面提高经济价值的观点相一致。该综述以均相催化剂的发展和应用为切入点,系统性地介绍了目前针对1,3-丁二烯的化工转化所采用的催化过程。通过对反应机理、催化剂进展、产业化应用等方面的综合分析,全面呈现了1,3-丁二烯在橡胶工业之外的主要化工转化途径,提供了全景式的描述。

See  Matthias Beller et al., https://doi.org/10.1039/D3IM00009E

  Back cover  

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本期封底文章来自华中科技大学冯光教授团队综述:Understanding the charging of supercapacitors by electrochemical quartz crystal microbalance。本图主要由右上角的超级电容器与中央的石英晶体芯片构成,展现了如何利用电化学石英晶体微天平(EQCM)来监测超级电容器的充放电过程。光束从电极-电解液界面由小到大至芯片处,代表EQCM对微观界面进行原位表征的能力。石英芯片从上至下由石英、金涂层和多孔涂覆电极这三部分构成,其上部离子与溶剂分子一起进入孔内代表EQCM可以对离子传输和溶剂化结构进行监测。图上橙色频率曲线和蓝色质量曲线则代表了该领域最重要的理论依据——Sauerbrey公式。该综述从EQCM发展历程、在超级电容器中的应用、与其他检测手段的结合等方面,介绍了EQCM在超级电容器领域内的重要进展。以此为基础讨论了离子交换类型和脱溶剂化程度对超级电容器性能的深刻影响,总结了EQCM的优点和缺点,对EQCM的下一步发展带来启示。

See Guang Feng et al., https://doi.org/10.1039/D2IM00038E

  • 本期内容

  01 Review | Page 155-174  

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Industrially applied and relevant transformations of 1,3-butadiene using homogeneous catalysts

Highlight: In this review, the use of 1,3-butadiene as a comparably cheap and abundant raw material to harvest fine and bulk chemicals is summarized in detail.

Citation: J. Yang, P. Wang, H. Neumann, R. Jackstell and M. Beller, Ind. Chem. Mater., 2023,1, 155-174.

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https://doi.org/10.1039/D3IM00009E


  02 Review | Page 175-187  

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Understanding the charging of supercapacitors by electrochemical quartz crystal microbalance

Highlight: Supercapacitors are highly valued energy storage devices and it's crucial to understand their charging mechanism. We present a comprehensive discussion on the applications of EQCM in the supercapacitor community.

Citation: L. Niu, L. Yang, J. Yang, M. Chen, L. Zeng, P. Duan, T. Wu, E. Pameté, V. Presser and G. Feng, Ind. Chem. Mater., 2023,1, 175-187.

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https://doi.org/10.1039/D2IM00038E


  03 Review | Page 188-206  

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Catalytic conversion network for lignocellulosic biomass valorization: a panoramic view

Highlight: The catalytic conversion networks for lignocellulose valorization including reaction routes, reaction types and key steps are comprehensively reviewed. The issues that need to be addressed for large-scale application are proposed.

Citation: S. Wang, A. Cheng, F. Liu, J. Zhang, T. Xia, X. Zeng, W. Fan and Y. Zhang, Ind. Chem. Mater., 2023,1, 188-206.

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https://doi.org/10.1039/D2IM00054G


  04 Review | Page 207-223  

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Perspective on oligomeric products from lignin depolymerization: their generation, identification, and further valorization

Highlight: A systematic summary on the current state-of-art of the formation, identification, and further valorization of oligomeric products during various lignin depolymerization processes.

Citation: Y. Han, B. A. Simmons and S. Singh, Ind. Chem. Mater., 2023,1, 207-223.

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https://doi.org/10.1039/D2IM00059H


  05 Review | Page 224-239  

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Ionic skin: from imitating natural skin to beyond

Highlight: The last decade has witnessed the birth and development of ionic skin. This article systematically reviews the research progress of ionic skin from the perspective of function.

Citation: Z. Chen and Y. Wang, Ind. Chem. Mater., 2023,1, 224-239.

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https://doi.org/10.1039/D2IM00062H


  06 Paper | Page 240-246  

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Understanding the interaction mechanism of carbazole/anthracene with N,N-dimethylformamide: NMR study substantiated carbazole separation

Highlight: In this work, the intermolecular interaction of carbazole/anthracene with DMF was investigated using various NMR techniques. More importantly, the intermolecular hydrogen bond between carbazole and DMF in the form of C[double bond, length as m-dash]O⋯H–N was proposed.

Citation: H. Cao, M. Dou, Z. Lyu, Y. Wang, C. M. Pedersen and Y. Qiao, Ind. Chem. Mater., 2023,1, 240-246.

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https://doi.org/10.1039/D2IM00020B


  07 Paper | Page 247-253  

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Preparation of yolk–shell urchin-like porous Co3O4/NiO@C microspheres with excellent lithium storage performance

Highlight: Yolk–shell urchin-like porous Co3O4/NiO@C microspheres were synthesized via solvothermal method and annealing treatment. A high reversible capacity of 502.7 mA h g−1 was maintained after 1000 cycles at 5 C, showing the long cycling stability.

Citation: L. Yu, Q. Yang, G. Zhu and R. Che, Ind. Chem. Mater., 2023,1, 247-253.

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https://doi.org/10.1039/D2IM00017B


  08 Paper | Page 254-261  

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Large-scale direct regeneration of LiFePO4@C based on spray drying

Highlight: We present a scalable, cost-effective closed-loop regeneration process of spent LiFePO4, including homogenization, spray drying and sintering. The regenerated LiFePO4 exhibits excellent electrochemical properties.

Citation: Y. Zou, J. Cao, H. Li, W. Wu, Y. Liang and J. Zhang, Ind. Chem. Mater., 2023,1, 254-261.

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https://doi.org/10.1039/D2IM00007E


  09 Paper | Page 262-270  

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Theoretical insights into NH3 absorption mechanisms with imidazolium-based protic ionic liquids

Highlight: NH3 absorption in [BIm][Tf2N] is governed by hydrogen bonds between NH3 and the protic site on the cation and considerable effects of anions due to their interaction with the protic site.

Citation: W. Tu, S. Zeng, Y. Bai, X. Zhang, H. Dong and X. Zhang, Ind. Chem. Mater., 2023,1, 262-270.

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https://doi.org/10.1039/D2IM00041E

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  • 期刊简介

Industrial Chemistry & Materials (ICM) 是中国科学院主管,中国科学院过程工程研究所主办,英国皇家化学会(RSC)全球出版发行的Open Access英文期刊,由中国科学院过程工程研究所张锁江院士担任主编。ICM 以化学、化工、材料为学科基础,以交叉为特色,以应用为导向,重点关注工业过程中化学问题、高端材料创制中过程科学的国际前沿和重大技术突破,致力于打造国际学术交流平台,成为具有重大国际影响力、引领工业化学与材料学科发展的国际一流期刊。ICM 现已开通全球投稿,目前对读者作者双向免费,欢迎广大科研工作者积极投稿、阅读和分享!

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中国科学院过程工程研究所/河南大学

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Maohong Fan                                           Chao Lu(吕超)

University of Wyoming,US                         郑州大学

Anja V. Mudring                                       Rong Sun(孙蓉)

Aarhus University,DK                                 深圳先进电子材料国际创新研究院 

Quanhong Yang(杨全红)                          Shouliang Yi

天津大学                                                     National Energy Technology Laboratory,US

Tierui Zhang(张铁锐)                                Xiangping Zhang(张香平)  

中国科学院理化技术研究所                          中国科学院过程工程研究所

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https://blog.sciencenet.cn/blog-3388879-1390267.html

上一篇:ICM论文 | 德国Matthias Beller院士团队:均相催化剂在1,3-丁二烯的化工转化中的应用
下一篇:ICM论文 | 中国科学院长春应化所邢巍&葛君杰团队: 质子交换膜燃料电池(PEMFC)非贵金属ORR催化剂研究进展
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