The oxide superconductors, particularly those recently discovered that are based on La(2)CuO(4), have a set of peculiarities that suggest a common, unique mechanism: they tend in every case to occur n...more
Yuan Cao, Valla Fatemi, Shiang Fang, Kenji Watanabe, Takashi Taniguchi, Efthimios Kaxiras, Pablo Jarillo-Herrero
2018, Nature - Article
The behaviour of strongly correlated materials, and in particular unconventional superconductors, has been studied extensively for decades, but is still not well understood. This lack of theoretical u...more
Y. Shimizu, K. Miyagawa, K. Kanoda, M. Maesato, G. Saito
2003, Physical Review Letters - Article
1H NMR and static susceptibility measurements have been performed in an organic Mott insulator with a nearly isotropic triangular lattice, kappa-(BEDT-TTF)2Cu2(CN)(3), which is a model system of frust...more
Quantum spin liquids may be considered 'quantum disordered' ground states of spin systems, in which zero-point fluctuations are so strong that they prevent conventional magnetic long-range o...more
Tian-Heng Han, Joel S. Helton, Shaoyan Chu, Daniel G. Nocera, Jose A. Rodriguez-Rivera, Collin Broholm, Young S. Lee
2012, Nature - Article
Neutron scattering measurements on single-crystal samples of the mineral herbertsmithite, which is a spin-1/2 kagome-lattice antiferromagnet, provide evidence of fractionalized spin excitations at low...more
A. Banerjee, C. A. Bridges, J.-Q. Yan, A. A. Aczel, L. Li, M. B. Stone, G. E. Granroth, M. D. Lumsden, Y. Yiu, J. Knolle, S. Bhattacharjee, D. L. Kovrizhin, R. Moessner, D. A. Tennant, D. G. Mandrus, S. E. Nagler
2016, Nature Materials - Article
Quantum spin liquids (QSLs) are topological states of matter exhibiting remarkable properties such as the capacity to protect quantum information from decoherence. Whereas their featureless ground sta...more
This is an introductory review of the physics of quantum spin liquid states. Quantum magnetism is a rapidly evolving field, and recent developments reveal that the ground states and low-energy physics...more
Z. Y. Meng, T. C. Lang, S. Wessel, F. F. Assaad, A. Muramatsu
2010, Nature - Article
At sufficiently low temperatures, condensed-matter systems tend to develop order. A notable exception to this behaviour is the case of quantum spin liquids, in which quantum fluctuations prevent a tra...more
Y. Kasahara, T. Ohnishi, Y. Mizukami, O. Tanaka, Sixiao Ma, K. Sugii, N. Kurita, H. Tanaka, J. Nasu, Y. Motome, T. Shibauchi, Y. Matsuda
2018, Nature - Article
The quantum Hall effect in two-dimensional electron gases involves the flow of topologically protected dissipationless charge currents along the edges of a sample. Integer or fractional electrical con...more
Arnab Banerjee, Jiaqiang Yan, Johannes Knolle, Craig A Bridges, Matthew B Stone, Mark D Lumsden, David G Mandrus, David A Tennant, Roderich Moessner, Stephen E Nagler
2017, Science - Article
The Kitaev quantum spin liquid (KQSL) is an exotic emergent state of matter exhibiting Majorana fermion and gauge flux excitations. The magnetic insulator α-RuCl3 is thought to realize a pr...more
Kate A. Ross, Lucile Savary, Bruce D. Gaulin, Leon Balents
2011, Physical Review X - Article
Recent work has highlighted remarkable effects of classical thermal fluctuations in the dipolar spin ice compounds, such as “artificial magnetostatics,” manifesting as Coulombic power-law spin correla...more
The quantum pyrochlore antiferromagnet is studied by perturbative expansions and exact diagonalization of small clusters. We find that the ground state is a spin-liquid state: The spin-spin correlatio...more
R. Coldea, D. A. Tennant, A. M. Tsvelik, Z. Tylczynski
2001, Physical Review Letters - Article
The ground-state ordering and dynamics of the two-dimensional S = 1/2 frustrated Heisenberg antiferromagnet Cs(2)CuCl(4) are explored using neutron scattering in high magnetic fields. We find that the...more
The nature of quantum spin liquids, a novel state of matter where strong quantum fluctuations destroy the long-range magnetic order even at zero temperature, is a long-standing issue in physics. We me...more
R. Islam, C. Senko, W. C. Campbell, S. Korenblit, J. Smith, A. Lee, E. E. Edwards, C.-C. J. Wang, J. K. Freericks, C. Monroe
2013, Science - Article
Frustration, or the competition between interacting components of a network, is often responsible for the emergent complexity of many-body systems. For instance, frustrated magnetism is a hallmark of ...more
T. Itou, A. Oyamada, S. Maegawa, M. Tamura, R. Kato
2008, Physical Review B - Article
The family of layered organic salts X[Pd(dmit)2]2 are Mott insulators and form scalene-triangular spin-1∕2 systems. Among them, EtMe3Sb[Pd(dmit)2]2 has a nearly regular-triangular lattice. We have inv...more
The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare-earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Spin ices ...more
Luke J Sandilands, Yao Tian, Kemp W Plumb, Young-June Kim, Kenneth S Burch
2015, Physical Review Letters - Article
The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid state...more
Low-temperature thermal-transport measurements of a frustrated organic magnet in which a quantum spin-liquid is believed to exist, suggest that the emergence of this state is accompanied by a spin-gap...more
Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in la...more
We perform highly accurate density matrix renormalization group (DMRG) simulations to investigate the ground-state properties of the spin-1/2 antiferromagnetic square lattice Heisenberg J1-J2 model. B...more
Hidenori Takagi, Tomohiro Takayama, George Jackeli, Giniyat Khaliullin, Stephen E. Nagler
2019, Nature Reviews Physics - Article
The Kitaev model is an exactly solvable S = 1/2 spin model on a 2D honeycomb lattice, in which the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the gr...more
Mingxuan Fu, Takashi Imai, Tian-Heng Han, Young S Lee
2015, Science - Article
The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. ...more
We present and discuss a variational approach to the one band Hubbard model in the limit of a large on-site Coulomb repulsion. The trial wavefunctions are the projected wavefunctions, generalized Gutz...more
We develop a nonperturbative gauge mean field theory (gMFT) method to study a general effective spin-1/2 model for magnetism in rare earth pyrochlores. gMFT is based on a novel exact slave-particle fo...more
J. Knolle, D. L. Kovrizhin, J. T. Chalker, R. Moessner
2014, Physical Review Letters - Article
We provide a complete and exact theoretical study of the dynamical structure factor of a two-dimensional quantum spin liquid in gapless and gapped phases, as realized in Kitaev’s honeycomb model. We s...more
S-H Baek, S-H Do, K-Y Choi, Y S Kwon, A U B Wolter, S Nishimoto, Jeroen van den Brink, B Büchner
2017, Physical Review Letters - Article
We report a ^{35}Cl nuclear magnetic resonance study in the honeycomb lattice α-RuCl_{3}, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our...more
Joseph A. M. Paddison, Marcus Daum, Zhiling Dun, Georg Ehlers, Yaohua Liu, Matthew B. Stone, Haidong Zhou, Martin Mourigal
2016, Nature Physics - Article
A detailed and systematic neutron-scattering study uncovers a continuum of magnetic excitations down to 0.06 K in the triangular quantum magnet YbMgGaO4 — an observation consistent with quantum spin l...more
C Broholm, R J Cava, S A Kivelson, D G Nocera, M R Norman, T Senthil
2020, Science - Article
Spin liquids are quantum phases of matter with a variety of unusual features arising from their topological character, including "fractionalization"-elementary excitations that behave as fra...more
I construct a Jordan-Wigner transformation for spin-one-half quantum systems on two-dimensional lattices. I show that the spin-one-half XY (i.e., a hard-core Bose system) is equivalent (on any two-dim...more
We consider the Kane-Mele model supplemented by a Hubbard U term. The phase diagram is mapped out using projective auxiliary field quantum Monte Carlo simulations. The quantum spin liquid of the Hubba...more
Yao Shen, Yao-Dong Li, Hongliang Wo, Yuesheng Li, Shoudong Shen, Bingying Pan, Qisi Wang, H. C. Walker, P. Steffens, M. Boehm, Yiqing Hao, D. L. Quintero-Castro, L. W. Harriger, M. D. Frontzek, Lijie Hao, Siqin Meng, Qingming Zhang, Gang Chen, Jun Zhao
2016, Nature - Article
A spin excitation continuum across a large region of the Brillouin zone that persists at near-zero temperatures provides evidence for a quantum spin liquid state with a spinon Fermi surface in YbMgGaO...more
2017, Annual Review of Condensed Matter Physics - Article
Quantum spin liquids have fascinated condensed matter physicists for decades because of their unusual properties such as spin fractionalization and long-range entanglement. Unlike conventional symmet...more
Yuesheng Li, Gang Chen, Wei Tong, Li Pi, Juanjuan Liu, Zhaorong Yang, Xiaoqun Wang, Qingming Zhang
2015, Physical Review Letters - Article
YbMgGaO4, a structurally perfect two-dimensional triangular lattice with an odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments for the Yb(3+) ions, is like...more
Arnab Banerjee, Paula Lampen-Kelley, Johannes Knolle, Christian Balz, Adam Anthony Aczel, Barry Winn, Yaohua Liu, Daniel Pajerowski, Jiaqiang Yan, Craig A. Bridges, Andrei T. Savici, Bryan C. Chakoumakos, Mark D. Lumsden, David Alan Tennant, Roderich Moessner, David G. Mandrus, Stephen E. Nagler
2018, npj Quantum Materials - Article
The celebrated Kitaev quantum spin liquid (QSL) is the paradigmatic example of a topological magnet with emergent excitations in the form of Majorana Fermions and gauge fluxes. Upon breaking of time-r...more
B. Fåk, E. Kermarrec, L. Messio, B. Bernu, C. Lhuillier, F. Bert, P. Mendels, B. Koteswararao, F. Bouquet, J. Ollivier, A. D. Hillier, A. Amato, R. H. Colman, A. S. Wills
2012, Physical Review Letters - Article
Magnetic susceptibility, NMR, muon spin relaxation, and inelastic neutron scattering measurements show that kapellasite, Cu3Zn(OH)6Cl2, a geometrically frustrated spin-1/2 kagome antiferromagnet polym...more
Abelian and non‐Abelian gauge theories are of central importance in many areas of physics. In condensed matter physics, Abelian U(1) lattice gauge theories arise in the description of certain quantum ...more
Masashige Matsumoto, B. Normand, T. M. Rice, Manfred Sigrist
2004, Physical Review B - Article
Thallium copper chloride is a quantum spin liquid of S=1/2 Cu2+ dimers. Interdimer superexchange interactions give a three-dimensional magnon dispersion and a spin gap significantly smaller than the d...moreCompass models: Theory and physical motivations
Zohar Nussinov, Jeroen van den Brink
2015, Reviews of Modern Physics - Article
Compass models are theories of matter in which the couplings between the internal spin (or other relevant field) components are inherently spatially (typically, direction) dependent. A simple illustra...more
L. Santos, M. A. Baranov, J. I. Cirac, H.-U. Everts, H. Fehrmann, M. Lewenstein
2004, Physical Review Letters - Article
We demonstrate the possibility of creating and controlling an ideal and trimerized optical Kagomé lattice, and study the low temperature physics of various atomic gases in such lattices. In the trimer...more
The physical description of all materials is rooted in quantum mechanics, which describes how atoms bond and electrons interact at a fundamental level. Although these quantum effects can in many cases...more
This review gives a rather general discussion of high temperature superconductors as an example of a strongly correlated material. The argument is made that in view of the many examples of unconventio...more
In frustrated magnetic systems, long-range ordering is forbidden and degeneracy of energy states persists, even at extremely low temperatures. Under certain conditions, these systems form an exotic qu...more
J. Nasu, J. Knolle, D. L. Kovrizhin, Y. Motome, R. Moessner
2016, Nature Physics - Article
An intriguing state of matter known as a quantum spin liquid has been predicted to host Majorana fermions. A detailed theoretical and numerical analysis re-interprets existing Raman data for α-RuCl3 a...more
S.-H. Lee, H. Kikuchi, Y. Qiu, B. Lake, Q. Huang, K. Habicht, K. Kiefer
2007, Nature Materials - Article
A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S=1/2), however, novel quantum paramagnetic states may appear. T...more
Ravi Yadav, Nikolay A. Bogdanov, Vamshi M. Katukuri, Satoshi Nishimoto, Jeroen van den Brink, Liviu Hozoi
2016, Scientific Reports - Article
Large anisotropic exchange in 5d and 4d oxides and halides open the door to new types of magnetic ground states and excitations, inconceivable a decade ago. A prominent case is the Kitaev spin liquid,...more
An effective low-energy Hamiltonian of itinerant electrons for iridium oxide Na2IrO3 is derived by an ab initio downfolding scheme. The model is then reduced to an effective spin model on a honeycomb ...more
Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in co...more
2017, Angewandte Chemie International Edition - Article
A highly crystalline copper(II) benzenehexathiolate coordination polymer (Cu-BHT) has been prepared. The two-dimensional kagome structure has been confirmed by powder X-ray diffraction, high-resolutio...more
The “spin-ice” state found in the rare-earth pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7 offers a beautiful realization of classical magnetostatics, complete with magnetic monopole excitations. It has be...more
We consider possible exotic ground states of quantum spin ice as realized in rare earth pyrochlores. Prior work [Savary and Balents, Phys. Rev. Lett. 108, 037202 (2012).PRLTAO0031-900710.1103/PhysRevL...more
Jiacheng Zheng, Kejing Ran, Tianrun Li, Jinghui Wang, Pengshuai Wang, Bin Liu, Zheng-Xin Liu, B Normand, Jinsheng Wen, Weiqiang Yu
2017, Physical Review Letters - Article
α-RuCl_{3} is a leading candidate material for the observation of physics related to the Kitaev quantum spin liquid (QSL). By combined susceptibility, specific-heat, and nuclear-magnetic-resonance mea...more
F. L. Pratt, P. J. Baker, S. J. Blundell, T. Lancaster, S. Ohira-Kawamura, C. Baines, Y. Shimizu, K. Kanoda, I. Watanabe, G. Saito
2011, Nature - Article
Characterization of a quantum spin liquidTheoretical predictions of the existence of an exotic state of matter called a quantum spin liquid have been supported by experimental evidence, but many funda...more